Insight into Hydrate Film Growth: Unusual Growth of Methane Hydrate Film at the Interface of Methane and the Aqueous Solution of Malonic Acid

Результат исследования: Научные публикации в периодических изданияхстатья

Аннотация

In this paper, we argue there is a new way of growing hydrate film other than two currently known ones, namely, a hydrate shell on the water surface without a surfactant and various hydrate dendrimers in the presence of surfactants. A previously unknown growth form of hydrate film occurs at the boundary between an aqueous solution of malonic acid and methane gas. These are gas-filled rounded bodies (like bubbles) of irregular shape which intergrow into the bulk aqueous phase. A possible phenomenological mechanism of the growth of these bodies is discussed. It is assumed such phenomena may take place in real systems during the formation of gas hydrates in water-in-oil dispersions.

Язык оригиналаанглийский
Страницы (с-по)1927-1934
Число страниц8
ЖурналCrystal Growth and Design
Том20
Номер выпуска3
DOI
СостояниеОпубликовано - 4 мар 2020

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