Design and performance of asymmetric supported membranes for oxygen and hydrogen separation

Vladislav A. Sadykov; Nikita F. Eremeev; Yulia E. Fedorova; Alexey V. Krasnov; Ludmilla N. Bobrova; Yulia N. Bespalko; Anton I. Lukashevich; Pavel I. Skriabin; Oleg L. Smorygo; Andre C. Van Veen

doi:10.1016/j.ijhydene.2020.01.106

Design and performance of asymmetric supported membranes for oxygen and hydrogen separation

Vladislav A. Sadykov, Nikita F. Eremeev, Yulia E. Fedorova, Alexey V. Krasnov, Ludmilla N. Bobrova, Yulia N. Bespalko, Anton I. Lukashevich, Pavel I. Skriabin, Oleg L. Smorygo, Andre C. Van Veen

Результат исследования: Научные публикации в периодических изданиях › статья › рецензирование

3 Цитирования (Scopus)

Аннотация

Producing syngas and hydrogen from biofuels is a promising technology in the modern energy. In this work results of authors’ research aimed at design of supported membranes for oxygen and hydrogen separation are reviewed. Nanocomposites were deposited as thin layers on Ni–Al foam substrates. Oxygen separation membranes were tested in CH₄ selective oxidation/oxi-dry reforming. The hydrogen separation membranes were tested in C₂H₅OH steam reforming. High oxygen/hydrogen fluxes were demonstrated. For oxygen separation membranes syngas yield and methane conversion increase with temperature and contact time. For reactor with hydrogen separation membrane a good performance in ethanol steam reforming was obtained. Hydrogen permeation increases with ethanol inlet concentration, then a slight decrease is observed. The results of tests demonstrated the oxygen/hydrogen permeability promising for the practical application, high catalytic performance and a good thermochemical stability.

Язык оригинала	английский
Страницы (с-по)	20222-20239
Число страниц	18
Журнал	International Journal of Hydrogen Energy
Том	46
Номер выпуска	38
DOI	https://doi.org/10.1016/j.ijhydene.2020.01.106
Состояние	Опубликовано - 3 июн. 2021

Предметные области OECD FOS+WOS

1.04 ХИМИЧЕСКИЕ НАУКИ
2.07 ЭНЕРГЕТИКА И РАЦИОНАЛЬНОЕ ПРИРОДОПОЛЬЗОВАНИЕ

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10.1016/j.ijhydene.2020.01.106

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Sadykov, V. A., Eremeev, N. F., Fedorova, Y. E., Krasnov, A. V., Bobrova, L. N., Bespalko, Y. N., Lukashevich, A. I., Skriabin, P. I., Smorygo, O. L., & Van Veen, A. C. (2021). Design and performance of asymmetric supported membranes for oxygen and hydrogen separation. International Journal of Hydrogen Energy, 46(38), 20222-20239. https://doi.org/10.1016/j.ijhydene.2020.01.106

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title = "Design and performance of asymmetric supported membranes for oxygen and hydrogen separation",

abstract = "Producing syngas and hydrogen from biofuels is a promising technology in the modern energy. In this work results of authors{\textquoteright} research aimed at design of supported membranes for oxygen and hydrogen separation are reviewed. Nanocomposites were deposited as thin layers on Ni–Al foam substrates. Oxygen separation membranes were tested in CH4 selective oxidation/oxi-dry reforming. The hydrogen separation membranes were tested in C2H5OH steam reforming. High oxygen/hydrogen fluxes were demonstrated. For oxygen separation membranes syngas yield and methane conversion increase with temperature and contact time. For reactor with hydrogen separation membrane a good performance in ethanol steam reforming was obtained. Hydrogen permeation increases with ethanol inlet concentration, then a slight decrease is observed. The results of tests demonstrated the oxygen/hydrogen permeability promising for the practical application, high catalytic performance and a good thermochemical stability.",

keywords = "Asymmetric supported membranes, Methane and ethanol reforming, Nanocomposites, Oxygen and hydrogen separation, Process parameters",

author = "Sadykov, {Vladislav A.} and Eremeev, {Nikita F.} and Fedorova, {Yulia E.} and Krasnov, {Alexey V.} and Bobrova, {Ludmilla N.} and Bespalko, {Yulia N.} and Lukashevich, {Anton I.} and Skriabin, {Pavel I.} and Smorygo, {Oleg L.} and {Van Veen}, {Andre C.}",

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month = jun,

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doi = "10.1016/j.ijhydene.2020.01.106",

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Design and performance of asymmetric supported membranes for oxygen and hydrogen separation. / Sadykov, Vladislav A.; Eremeev, Nikita F.; Fedorova, Yulia E. и др.

В: International Journal of Hydrogen Energy, Том 46, № 38, 03.06.2021, стр. 20222-20239.

Результат исследования: Научные публикации в периодических изданиях › статья › рецензирование

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T1 - Design and performance of asymmetric supported membranes for oxygen and hydrogen separation

AU - Sadykov, Vladislav A.

AU - Eremeev, Nikita F.

AU - Fedorova, Yulia E.

AU - Krasnov, Alexey V.

AU - Bobrova, Ludmilla N.

AU - Bespalko, Yulia N.

AU - Lukashevich, Anton I.

AU - Skriabin, Pavel I.

AU - Smorygo, Oleg L.

AU - Van Veen, Andre C.

PY - 2021/6/3

Y1 - 2021/6/3

N2 - Producing syngas and hydrogen from biofuels is a promising technology in the modern energy. In this work results of authors’ research aimed at design of supported membranes for oxygen and hydrogen separation are reviewed. Nanocomposites were deposited as thin layers on Ni–Al foam substrates. Oxygen separation membranes were tested in CH4 selective oxidation/oxi-dry reforming. The hydrogen separation membranes were tested in C2H5OH steam reforming. High oxygen/hydrogen fluxes were demonstrated. For oxygen separation membranes syngas yield and methane conversion increase with temperature and contact time. For reactor with hydrogen separation membrane a good performance in ethanol steam reforming was obtained. Hydrogen permeation increases with ethanol inlet concentration, then a slight decrease is observed. The results of tests demonstrated the oxygen/hydrogen permeability promising for the practical application, high catalytic performance and a good thermochemical stability.

AB - Producing syngas and hydrogen from biofuels is a promising technology in the modern energy. In this work results of authors’ research aimed at design of supported membranes for oxygen and hydrogen separation are reviewed. Nanocomposites were deposited as thin layers on Ni–Al foam substrates. Oxygen separation membranes were tested in CH4 selective oxidation/oxi-dry reforming. The hydrogen separation membranes were tested in C2H5OH steam reforming. High oxygen/hydrogen fluxes were demonstrated. For oxygen separation membranes syngas yield and methane conversion increase with temperature and contact time. For reactor with hydrogen separation membrane a good performance in ethanol steam reforming was obtained. Hydrogen permeation increases with ethanol inlet concentration, then a slight decrease is observed. The results of tests demonstrated the oxygen/hydrogen permeability promising for the practical application, high catalytic performance and a good thermochemical stability.

KW - Asymmetric supported membranes

KW - Methane and ethanol reforming

KW - Nanocomposites

KW - Oxygen and hydrogen separation

KW - Process parameters

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